Evidently the Apollo 11 team were the most profligate litterers in history (up to then), according to this article from the July 20, 1969 Bartlesville Examiner-Enterprise.
Many folks of this vintage will immediately think of the jingle "Please, please, don't be a litterbug / 'Cause ev'ry litter bit hurts!" You can hear it at the very end of this 1961 PSA:
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